Despite enormous efforts by many research groups, Sr2IrO4 was found to stay remarkably insulating in thin film form. Now, a high-pressure oxygen annealing treatment on the Sr2IrO4 thin film realized the long-sought metallicity for the first time. An emerging transport phase diagram was deduced from the experiment that features an interplay between two states: the robust insulating state, which is likely dominated by the defect scattering effect of planar oxygen vacancies O(2), and the new metallic state, which likely reflects an intrinsic bulk-like property of the IrO2 planes with effective electron doping due to apical oxygen vacancies O(1).
- Zhen Song
- You-Shan Zhang
- Rui-Hua He